Complexes of Re2(O2C2H3)Cl2*2H2O with 1 9-Diethyladenine

Poster Number

11

Format

Poster Presentation

Abstract/Artist Statement

Dimetal carboxylate compounds are proposed to exhibit antitumor activity by reacting with DNA nucleobases. Dirhenium complexes containing a cis-carboxylate core similar to Re2(O2C2H3)2Cl4·2H2O show anticancer properties. These complexes are known to preferentially bind to the purine nucleobases adenine and guanine. To model this reaction, Re2(O2C2H3)2Cl4·2H2O was reacted with a model adenine compound, 1,9- diethyladenine, which is isolated as an iodide salt. Anion exchange reactions were carried out to replace the iodide with different anions (PF6-, BF4-, BPh4-). These salts were reacted with the dirhenium compound, Re2(O2C2H3)2Cl4·2H2O, and the green products were isolated and characterized. UV/visible, IR, and 1H NMR spectroscopic results will be presented.

Location

Pacific Geosciences Center

Start Date

30-4-2005 1:00 PM

End Date

30-4-2005 3:00 PM

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Apr 30th, 1:00 PM Apr 30th, 3:00 PM

Complexes of Re2(O2C2H3)Cl2*2H2O with 1 9-Diethyladenine

Pacific Geosciences Center

Dimetal carboxylate compounds are proposed to exhibit antitumor activity by reacting with DNA nucleobases. Dirhenium complexes containing a cis-carboxylate core similar to Re2(O2C2H3)2Cl4·2H2O show anticancer properties. These complexes are known to preferentially bind to the purine nucleobases adenine and guanine. To model this reaction, Re2(O2C2H3)2Cl4·2H2O was reacted with a model adenine compound, 1,9- diethyladenine, which is isolated as an iodide salt. Anion exchange reactions were carried out to replace the iodide with different anions (PF6-, BF4-, BPh4-). These salts were reacted with the dirhenium compound, Re2(O2C2H3)2Cl4·2H2O, and the green products were isolated and characterized. UV/visible, IR, and 1H NMR spectroscopic results will be presented.